Summary and Conclusions

We measured dendritic growth velocities and tip radii of curvature of succinonitrile in microgravity using the IDGE instrument flown in low-earth orbit. The on-orbit data, when compared to terrestrial dendritic growth data obtained using the same apparatus and techniques, demonstrate that: 1) convective effects under terrestrial conditions cause growth speed increases to a factor of 2 at the lower supercoolings ( DeltaT < 0.5 K), and convection effects remain discernible under terrestrial conditions up to supercoolings as high as 1.7 K. 2) In the supercooling range above 0.47 K, microgravity data remain virtually free of convective or chamber effects, and may be used reliably for examining diffusion-limited dendritic growth theories. 3) A diffusion solution to the dendrite problem, combined with a unique scaling constant, sigma*, fails to yield accuratepredictions of the growth velocity and dendritic tip radii. 4) Growth Péclet numbers calculated from Ivantsov s solution deviate systematically from the IDGE data observed under diffusion-limited conditions. 5) The scaling parameter sigma* does not appear to be a constant independent ofsupercooling. Finally, 6), the sigma* measurements from the terrestrial and microgravity data are ingood agreement with each other, despite a difference of over six orders of magnitude in the quasi-static acceleration environment of low-earth orbit and terrestrial conditions.

The most important of these findings is that Ivantsov s description of the conduction of latent heat from adendrite needs to be modified in order to describe the growth of SCN dendrites accurately. We offer here one key observation: the diffusion field of the Ivantsov formulation is based on a steady-state dendrite which is a paraboloid of revolution. But we know from our own measurements and others, that neither assumption is true [Huang, 1981][Koss, 1995]. The microgravity data reported here in the diffusion limited regime should help to constrains the possibilities for theoretical modeling. Diffusion-limited growth data can serve as a benchmark for testing and developing theories and provide a better basis for phenomenological models of dendritic growth kinetics. The publication of our dendritic growth data in tabular form is meant to facilitate such studies. The data from our recent microgravity experiment will be added to this as soon as it is available.