This used to be the Title for Frequently Asked Questions
(and now it's just a title for a lowly chart)

Generalized Rules for Gas Permeability
Here is a reproduction of that chart that I mentioned, originally written up by Freidlander and Rickles.
Essentially, it lists principal variables and how they effect gas permeation rate.
Temperature
- Arrhenius-type effect - for permanent and other small size gases
- Activation Energy is function of temperature for CO2 and H20 above glass temperature
- Arrhenius-type effect foes not hold for organics
Pressure, Concentration
- For permanent gases and CO2, independent of pressure
- For most other gases, permeability is a function of pressure
Penetrant nature
- Permeability is a decreasing function of molecular diameter
- Mutual compatibility and ease of condensation increases permeability
Plasticizing effect
- Ability to plasticize increases permeability
Polymer structure
- Crystalling region acts as an impermeable phase so rates are proportional to volume fraction of amorphous phase
- Thermal and mechanical working history is important
- Solvent conditioning is important
- Cross linking reduces diffusion rates
Grafting
- Grafting greatly affects permeability
Irradiation
- Irradiation causes cross-linking, which reduces diffusion
Film Thickness
- Usually has no effect, but may be important for very thin films or for films with large concentration gradients.